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Ozone Production from Biomass Burning in the Amazon: Preliminary WRF-Chem Simulations and Comparison with In-Situ Data from the CO-CLAIM Experiment. M. M. Bela 1 , K. M. Longo 2 , S. R. Freitas 2 , P. Artaxo 1 1 Institute of Physics, University of S ã o Paulo
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Ozone Production from Biomass Burning in the Amazon: Preliminary WRF-Chem Simulations and Comparison with In-Situ Data from the CO-CLAIM Experiment M. M. Bela1, K. M. Longo2, S. R. Freitas2, P. Artaxo1 1Institute of Physics, University of São Paulo 2Center for Weather Forecasting and Climate Studies (CPTEC), National Institute for Space Research (INPE)
Objectives Identify Ozone Production Regimes in the Amazon Validate/Compare WRF-Chem / CCATT-BRAMS Test Model Sensitivity to Emissions Improve South American Air Quality Forecasting Context Data Emissions Simulations Conclusions
Amazonian Biomass Burning Global biomass burning: 70% of BC SW direct radiative forcing [Chin 2002] Amazon deforestation: 70% of Brazil’s CO2 emissions [INPA] Wet Season Burning Season Source: Paulo Artaxo Context Data Emissions Simulations Conclusions
Ozone Production and Transport Nox + VOCs + H2O + T -> O3 Vertical transport by deep convection Longitudinal transport by high-level winds São Paulo Source: Saulo Freitas Context Data Emissions Simulations Conclusions
Ozone Production and Transport Dry deposition of ozone (1.e-3 kg/m^2)(Accum. 2 months 00Z30SEP2002) Precursors emission area Downwind formation and deposition São Paulo Source: Karla Longo Context Data Emissions Simulations Conclusions
CO-CLAIM Experiment . Manaus Southern Amazon burning season 10-21 October 2007 Ozone measurements (1s) on 8 flights Alta Floresta . Context Data Emissions Simulations Conclusions
Ozone Data Context Data Emissions Simulations Conclusions
Model Setup WRF-Chem 3.0.1 40km, 136x168, 1-23 Oct. 2007 Timestep: 200s (met), 600s (chem) ICs/BCs: ECMWF (met), idealized profile (chem) Chemistry: RACM-GOCART Radiation: RRTM (longwave), Goddard (shortwave) Land-Surface Model: Noah Microphysics: 5-class mixed-phase Cumulus: Grell-Devenyi ensemble Context Data Emissions Simulations Conclusions
Emissions Data Fire Product (DSA, ABBA) CO Emissions [mol/km^2-hr] Fire pixels from remote sensing fire products (GOES-8 WF_ABBA, INPE_AVHRR, MODIS) weighted by vegetation type burning emissions factors [Longo and Freitas, 2006]. 40km domain 10km domain Context Data Emissions Simulations Conclusions
Model Results Context Data Emissions Simulations Conclusions
Future Work Improve Model Initial and Boundary Conditions Land-Surface: High-Resolution Land Data Assimilation Chemistry: Global Model Context Data Emissions Simulations Conclusions
More Future Work Model Validation with Meteorological Data 10km / 1km two-way nesting Comparisons with CCATT-BRAMS Clean Case: LBA-BARCA (November 2008) Context Data Emissions Simulations Conclusions
Obrigada! Fulbright Commission Brazil Steven Peckham, Georg Grell (NOAA/FSL) Rafael Mello, Rafael Stockler Marcelo Alonso (CPTEC-INPE) Maria da Fatima Andrade, Marcio Gledson, Pedro Pais Lopes (IAG-USP)