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New Instruments for Neutrino Relics and Mass CERN, 8 December 2008

New Instruments for Neutrino Relics and Mass CERN, 8 December 2008. Orbital Electron-Capture Decay of Stored and Cooled Hydrogen-like Ions in the Experimental Storage Ring, ESR. Christophor Kozhuharov, GSI Darmstadt Outline: Motivation

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New Instruments for Neutrino Relics and Mass CERN, 8 December 2008

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  1. New Instruments for Neutrino Relics and Mass CERN, 8 December 2008 Orbital Electron-Capture Decay of Stored and Cooled Hydrogen-like Ions in the Experimental Storage Ring, ESR • Christophor Kozhuharov, GSI Darmstadt • Outline: • Motivation • Production, separation, storage, cooling, and nondestructive detecting of highly-charged radioactive ions at the FRS-ESR complex • Two-body electron-capture decay of highly-charged ions. • Single-ion decay spectroscopy • Experimental results for EC of H-like 140Pr and 142Pm ions • Some hypotheses on the observed non-exponential decay

  2. FRS/ESR Mass-and-Lifetime Collaboration G. Audi, K. Beckert, P. Beller†, F. Bosch, D. Boutin, C. Brandau, Th. Bürvenich,L. Chen, I. Cullen, Ch. Dimopoulou, H. Essel, B. Fabian, Th. Faestermann, B. Franczak, B. Franzke, H. Geissel, E. Haettner, M. Hausmann, S. Hess, P. Kienle, O. Klepper, H.-J. Kluge, C. Kozhuharov, R. Knöbel, J. Kurcewicz, S.A. Litvinov,Yu. A. Litvinov, Z. Liu, L. Maier,M. Mazzocco, F. Montes, A. Musumarra, G. Münzenberg, S. Nakajima, C. Nociforo, F. Nolden, Yu. N. Novikov, T. Ohtsubo, A. Ozawa, Z. Patyk, B. Pfeiffer, W. R. Plass, Z. Podolyak, M. Portillo, A. Prochazka, R. Reuschl, H. Schatz, Ch. Scheidenberger, M. Shindo, V. Shishkin, U. Spillmann, M. Steck, Th. Stöhlker, K. Sümmerer, B. Sun, K. Suzuki, K. Takahashi, S. Torilov, M. B. Trzhaskovskaya, S. Typel, D. J. Vieira, G. Vorobjev, P.M. Walker, H. Weick, S. Williams, M. Winkler,N. Winckler, D. Winters, H. Wollnik, T. Yamaguchi Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  3. Bound-State β-Decay M. Jung et al. Phys. Rev. Lett. 69 (1992) 2164 Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  4. Two-body β-decay of highly-charged ions Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  5. Secondary Beams of Short-Lived Nuclei Storage Ring ESR Linear Accelerator UNILAC Fragment Separator FRS Heavy-Ion Synchrotron SIS Production target Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  6. Production & Separation of Exotic Nuclei Highly-Charged Ions In-Flight separation Cocktail or one single nuclear species ≈ 600 MeV/u primary beams 400 MeV/u stored beams: fragments e.c. 140Pr, 142Pm, 205Hg, 207Tl, 206Tl, 122I

  7. Experimental Storage Ring, ESR: 108.4 m, 10-11 mbar Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  8. Stochastic cooling at the ESR Long. Kicker Transv. Pick-up Combiner Station Transv. Kicker ESR storage ring Long. Pick-up Stochastic cooling is particularly efficient for hot ion beams (Fixed energy: 400 MeV/u) Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  9. Cooling, i.e. enhancing the phase space density at constant beam velocities Electron cooling: G. Budker, 1967 Novosibirsk The momentum exchange of the ions with the cold collinear e- beam leads to an excellent emittance Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  10. 'Phase transition' to a linear ion chain ESR circumference ≈ 104 cm For 1000 stored ions, the mean distance amounts to about 10 cm. At mean distances of about 10 cm and larger the intra-beam-scatteringdisappears. M. Steck et al., PRL 77, 3803 (1996) Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  11. Recording the Schottky-noise Real time analyzer Sony-Tektronix 3066 ____________________________ 128 msec →FFT 64 msec_____________________ → FFT

  12. time SMS 4 particles with different m/q

  13. Sin(w1) Sin(w2) w4 w3 w2 w1 Sin(w3) time Sin(w4) SMS Fast Fourier Transform Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  14. 300 kHz / 60 MHz Schottky TCAP

  15. Orbital EC-experiments, decay schemes Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  16. Well-defined quantum states for parent and daughter ions I Well-defined states: → bare, 1, 2.. e- II Quasi 'free': → storage ring/ trap III Time-resolved decay: → single ions IV Correlated decay: → change of mass Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  17. Cooling at ESR David Boutin, PhD Thesis, Univ. Giessen, 2005 Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  18. Two-body beta decay f scales as m/q q does not change for the two-body β decay f changes only if the mass changes, or if the B-field changes. 260 Hz Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  19. EC in Hydrogen-like Ions Expectations: lb+/lEC (neutral atom) ≈1 lEC(H-like)/lEC(He-like) ≈ 0.5 FRS-ESR Experiment l(neutral)= 0.00341(1) s-1 G.Audi et al., NPA729 (2003) 3 lb+(bare) = 0.00158(8) s-1 (decay of 140Pr59+) lEC(H-like) = 0.00219(6) s-1 (decay of 140Pr58+) lEC(He-like) = 0.00147(7) s-1 (decay of 140Pr57+) lEC(H-like)/lEC(He-like) = 1.49(8) Yu. A. Litvinov et al., PRL 99, 262501 (2007) Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  20. Electron Capture in Hydrogen-like Ions Gamow-Teller transition 1+  0+ S. Typel and L. Grigorenko µ = +2.7812 µN (calc.) Theory: Z. Patyk et al., PR C77, 014306 (2008) The H-like ion decays by 20% faster than the neutral atom! Probability of EC Decay Neutral 140Pr: P = 2.381 He-like 140Pr: P = 2 λ(H)/λ(He) = (2I+1)/(2F+1) H-like 140Pr: P = 3 Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  21. Nuclear Decay of Stored Single Ions Time/channel = 30 sec. Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  22. We restrict the analysis to 1 to 3 injected ions: 1. The Schottky areas have a very large variance. 2. The variance of the amplitudes is larger than the step 3→4. 3. Problem of 'delayed cooling' Daughter Amplitude Amplitude Mother N. Winckler Amplitude distributions corresponding to 1,2,3-particles; 1 frame = 128 msec. The final data occur within +- 400 msec. in both the computer as well as in the ‘manual’ evaluations; In all cases the ‘appearance’ time has been taken into account.

  23. Examples of measured time-frequency traces ↕ Time/ch. = 640 msec Time/ch. = 640 ms Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  24. ↕ Time/ch. = 64 msec 2 140Pr58+ 1 140Pr58+ 1 140Ce58+ Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  25. Properties of measured time↔frequency traces 1. Continuous observation 2. Parent/daughter correlation 3. Detection of all EC decays 4. Delay between decay and "appearance" due to cooling 5. 140Pr: ER = 44 eV Delay: 900 (300) msec 142Pm: ER = 90 eV Delay: 1400 (400) msec from measured frequency:→p transformed to n (hadronic vertex) → bound e- annihilated (leptonic vertex) → ν created at td as νe = a │ν1 > + b ν2 > if conservation of lepton number holds Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  26. 2. Experimental results for EC of H-like ions: 140Pr58+ Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  27. Fast Fourier Transform of the data of 1.+2. run Frequency peak at f = 0.142 Hz Yu. A. Litvinov et al., Phys. Lett. B 664, 124 (2008) Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  28. 140Pr58+all runs: 2650 EC-decays from 7102 injections Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  29. 142Pm60+: 2740 EC decays from 7011 injections Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  30. 142Pm60+: zoom on the first 33 s after injection Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  31. Fits with pure exponential (1) and superimposed oscillation (2) • dNEC (t)/dt = N0 exp {- λt} λEC ; λ = λβ+ + λEC + λloss (1) • dNEC (t)/dt = N0 exp {- λt} λEC(t); λEC(t) = λEC [1+a cos(ωt+φ)](2) T = 7.06 (8) s φ = 0.4 (4) a = 0.18 (3) T = 7.10 (22) s φ = - 1.6 (4) a = 0.23 (4) Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  32. 3.Some hypotheses on the non-exponential decays Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  33. EC in H-like ions for nuclear g.s. → g.s. transitions Decay identified by correlatedchange of atomic mass at time td Different delay due to emission characteristics of the neutrino Small total line width(s) Ћ / ΔtObs (≈ 0.1 s ) ≈ 10 -14 eV >>Ћ /T (≈ 7 s) ≈ 10 -16 eV No third particle involved → daughter nucleus and neutrino entangled by momentum- and energy conservation → EPR scenario Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  34. Quantum beats from the hyperfine states ? Coherent excitation of the 1s hyperfine states F =1/2 & F=3/2Beat period T = h/ΔE ≈ 10-15 s µ = +2.7812 µN (calc.) Decay can occur only from the F=1/2 (ground) state Periodic spin flip to "sterile" F=3/2 ? → λEC reduced Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  35. "Classical" quantum beats Coherent excitation of an electron in two quantum states, separated by ΔE at time t0, e.g. 3P0 and 3P2 Observation of the decay photon(s) as a function of (t-t0) Exponential decay modulated by cos(ΔE / Ћ (t-t0)) -Δτ - if Δτ<< T = h/ΔE → no informationwhether E1 or E2 "which path"? addition ofamplitudes Chow et al., PR A11(1975) 1380 Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  36. Beats due to neutrino being not a mass eigenstate? The electron neutrino appears as coherent superposition of mass eigenstates The recoils appear as coherent superpositions of states entangled with the electron neutrino mass eigenstates by momentum- and energy conservation M + p12/2M + E1 = E M + p22/2M + E2 = E "Asymptotic" conservation of E, p E, p = 0 (c.m.) νe (mi, pi, Ei) M, pi2/2M m12 – m22 = Δ2m = 8 · 10-5 eV2 E1 – E2 = ΔEν ΔEν ≈ Δ2m/2M = 3.1 · 10-16 eV Δpν ≈ - Δ2m/ 2 <pν> = 2.0 · 10-11 eV Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  37. cos (ΔE/ћ t) with Tlab = h γ / ΔE ≈ 7s • a) M = 140 amu, Eν = 3.39 MeV (Pr) • b) M = 142 amu, Eν = 4.87 MeV (Pm) • M =141 amu, γ = 1.43, Δ2m12 = 8 · 10-5 eV2 • ΔE = hγ/ Tlab = 8.4 · 10 -16 eV • ΔEν = Δ2m /2 M = 3.1 · 10 -16 eV Christophor Kozhuharov, GSI Darmstadt EC-Decay of H-Like Ions

  38. New Experiment on 118Sb (122I)

  39. Decay scheme of 118Sb Experiment was scheduled: 31.07.2008-18.08.2008

  40. Decay scheme of 122I

  41. Decay statistics Correlations: 10.808 injections ~1080 EC-decays Many ions: 5718 injections ~5000 EC-decays Analyzed : I. About 60% of the overall data II. About 20% of the overall data Automatic analysis is delayed

  42. For the two-body EC decays of H-like 140Pr and 142Pm periodic modulations according to e –λt [1+a cos(ωt+φ)] with Tlab = 2π/ω = 7s, a ≈ 0.20 (4) were found • Statistical fluctuations are not excluded on a c.l. > 3.5 σ • Oscillation period T proportional to nuclear mass M ?

  43. Only a few out of many remaining questions • 1. Are the oscillations real ? → still modest statistics • 2. Can the coherence be maintained over some 10 s • keeping in mind the confinement in an electromagneticpotential, the continuous interaction, and thecontinuous observation ?? • How can we improve the statistics, what other systems can we probe,what other ESR settings can we use?

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